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Dynamical nuclear decoupling of electron spins in molecular graphenoid radicals and biradicals

Abstract:

We investigate the mechanisms of nuclear decoupling in synthetically-tailored graphenenoids, where the electron spin state is introduced by topological manipulation of the lattice. We compare molecular graphenoids containing one and two spin centres, introduced by pentagonal rings in the honeycomb lattice. Exploiting the molecular nature of the systems, we investigate the role of different nuclear species and environments. Variations on the Carr-Purcell-Meiboom-Gill pulse trains are used to p...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevB.101.094406

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Sub department:
Materials
Role:
Author
ORCID:
0000-0001-7488-6893
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
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Publisher:
American Physical Society Publisher's website
Journal:
Physical Review B Journal website
Volume:
101
Article number:
094406
Publication date:
2020-03-03
Acceptance date:
2020-02-13
DOI:
EISSN:
2469-9969
ISSN:
2469-9950
Language:
English
Keywords:
Pubs id:
1087346
Local pid:
pubs:1087346
Deposit date:
2020-02-13

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