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Anion-templated assembly of pseudorotaxanes: importance of anion template, strength of ion-pair thread association, and macrocycle ring size.

Abstract:

A wide range of pseudorotaxane assemblies containing positively charged pyridinium, pyridinium nicotinamide, imidazolium, benzimidazolium and guanidinium threading components, and macrocyclic isophthalamide polyether ligands have been prepared using a general anion templation procedure. In noncompetitive solvent media, coupling halide anion recognition by a macrocyclic ligand with ion-pairing between the halide anion and a strongly associated cation provides the driving force for interpenetra...

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Publication status:
Published

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Publisher copy:
10.1021/ja046278z

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
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Journal:
Journal of the American Chemical Society
Volume:
127
Issue:
7
Pages:
2292-2302
Publication date:
2005-02-01
DOI:
EISSN:
1520-5126
ISSN:
0002-7863
Source identifiers:
32997
Language:
English
Pubs id:
pubs:32997
UUID:
uuid:373f7f60-f56c-41c1-b8e4-0b662d1fa24c
Local pid:
pubs:32997
Deposit date:
2012-12-19

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