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Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom

Abstract:

Due to its element and site specificity, inner-shell photoelectron spectroscopy is a widely used technique to probe the chemical structure of matter. Here, we show that time-resolved inner-shell photoelectron spectroscopy can be employed to observe ultrafast chemical reactions and the electronic response to the nuclear motion with high sensitivity. The ultraviolet dissociation of iodomethane ( CH 3 I ) is investigated by ionization above the iodine 4 d edge, using time-resolved inner-shell ...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevA.97.043429

Authors


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Funding agency for:
Brouard, M
Grant:
FP7 EU People ITN project 238671
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Funding agency for:
Brouard, M
Grant:
FP7 EU People ITN project 238671
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Funding agency for:
Mackenzie, S
Grant:
EP/G00224X/1
EP/L005913/1
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Funding agency for:
Vallance, C
Grant:
EP/L005913/1
EP/G00224X/1
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Grant:
PNPASaward
amini-IPSgrant(ST/J002895/1
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Publisher:
American Physical Society Publisher's website
Journal:
Physical Review A Journal website
Volume:
97
Issue:
4
Article number:
043429
Publication date:
2018-04-27
Acceptance date:
2018-02-23
DOI:
EISSN:
2469-9934
ISSN:
2469-9926
Source identifiers:
848177
Pubs id:
pubs:848177
UUID:
uuid:41dffd66-9c8e-4cad-a1cf-d52a51f1e7dd
Local pid:
pubs:848177
Deposit date:
2018-05-19

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