Journal article
Effects of Coadsorbed Oxygen on the Infrared Driven Decomposition of N2O on Isolated Rh-5(+) Clusters
- Abstract:
-
The thermally induced decomposition of nitrous oxide on isolated Rh 5+ and Rh 5O + clusters has been investigated using mid-infrared multiple photon dissociation spectroscopy. The presence of a single coadsorbed oxygen atom is observed to have a profound effect on the cluster surface processes that ensue following infrared heating of the cluster. Exciting the infrared active N 2O bending transition in Rh 5N 2O + results predominantly (≥85%) in molecular desorption of the N 2O moiety, while th...
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- Publication status:
- Published
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- Publisher copy:
- 10.1021/jz2012963
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Bibliographic Details
- Journal:
- JOURNAL OF PHYSICAL CHEMISTRY LETTERS
- Volume:
- 2
- Issue:
- 24
- Pages:
- 3053-3057
- Publication date:
- 2011-12-15
- DOI:
- EISSN:
-
1948-7185
- ISSN:
-
1948-7185
- Source identifiers:
-
239921
Item Description
- Pubs id:
-
pubs:239921
- UUID:
-
uuid:66c2d236-c561-48aa-8601-d67e4468de69
- Local pid:
- pubs:239921
- Deposit date:
- 2012-12-19
Terms of use
- Copyright date:
- 2011
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