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Velocity-map imaging study of the photodissociation of acetaldehyde

Abstract:

Velocity-map imaging studies are reported for the photodissociation of acetaldehyde over a range of photolysis wavelengths s317.5–282.5 nmd. Images are obtained for both the HCO and CH3 fragments. The mean rotational energy of both fragments increases with photodissociation energy, with a lesser degree of excitation in the CH3 fragment. The CH3 images demonstrate that the CH3 fragments are rotationally aligned with respect to the recoil direction and this is interpreted, and well modeled, on ...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1063/1.1861886

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Institution:
University of Oxford
Role:
Author
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Institution:
University of Oxford
Role:
Author
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Funding agency for:
T P Softley
Grant:
Portfolio Partnership Grant No.GR/S71750/01
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Funding agency for:
H A Cruse
Grant:
Portfolio Partnership Grant No.GR/S71750/01
Publisher:
American Institute of Physics Publisher's website
Journal:
Journal of Chemical Physics Journal website
Volume:
122
Issue:
12
Pages:
124303 (13 pages)
DOI:
ISSN:
0021-9606
Language:
English
Subjects:
UUID:
uuid:670c66db-d2b6-4896-b7ad-a5da87199e06
Local pid:
ora:938
Deposit date:
2008-03-14

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