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Molecular aluminum hydrides identified by inelastic neutron scattering during H2 regeneration of catalyst-doped NaAlH2

Abstract:

Catalyst-doped sodium aluminum hydrides have been intensively studied as solid hydrogen carriers for onboard proton-exchange membrane (PEM) fuel cells. Although the importance of catalyst choice in enhancing kinetics for both hydrogen uptake and release of this hydride material has long been recognized, the nature of the active species and the mechanism of catalytic action are unclear. We have shown by inelastic neutron scattering (INS) spectroscopy that a volatile molecular aluminum hydride ...

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Publisher copy:
10.1021/jp055238u

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Journal:
Journal of Physical Chemistry B
Volume:
110
Issue:
2
Pages:
711-715
Publication date:
2006-01-19
DOI:
ISSN:
1520-6106
Source identifiers:
180215
Language:
English
Pubs id:
pubs:180215
UUID:
uuid:72bfad89-deb0-4224-9ec9-703326916dd1
Local pid:
pubs:180215
Deposit date:
2013-02-20

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