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A hydrogen fuel cell for rapid, enzyme-catalysed organic synthesis with continuous monitoring

Abstract:
A one-pot fuel cell for specific, enzyme-catalysed organic synthesis, with continuous monitoring of rate and reaction progress, combines an electrode catalysing rapid, reversible and diffusion-controlled interconversion of NADP+ and NADPH with a Pt electrode catalysing 2H+/H2 interconversion. This Communication demonstrates its performance and characteristics using the reductive amination of 2-oxoglutarate as a test system.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/c7cc08859k

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
ORCID:
0000-0002-0331-916X
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
ORCID:
0000-0003-0604-7670
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Oxford college:
St John's College
Role:
Author
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Chemical Communications Journal website
Volume:
54
Issue:
8
Pages:
972-975
Publication date:
2018-01-10
Acceptance date:
2018-01-02
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Pmid:
29319070
Source identifiers:
817803
Language:
English
Pubs id:
pubs:817803
UUID:
uuid:9e594836-1939-4bac-b4b5-fb1811f0a6b9
Local pid:
pubs:817803
Deposit date:
2019-03-06

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