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Journal article

Total synthesis of the Schisandraceae nortriterpenoid rubriflordilactone A

Abstract:

Full details of the total synthesis of the Schisandraceae nortriterpenoid natural product rubriflordilactone A are reported. Palladium- and cobalt-catalyzed polycyclizations were employed as key strategies to construct the central pentasubstituted arene from bromoendiyne and triyne precursors. This required the independent assembly of two AB ring aldehydes for combination with a common diyne component. A number of model systems were explored to investigate these two methodologies, and also to...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1002/chem.201703229

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Institution:
University of Oxford
Oxford college:
Jesus College
Role:
Author
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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
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Grant:
Marie Skłodowska-Curie actions for an Individual Fellowship (GC, GA N° 656012
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Grant:
additionalfunding(EP/K005391/1
AdvancedResearchFellowship (EAA)(EP/E055273/1)
Publisher:
Wiley Publisher's website
Journal:
Chemistry Journal website
Volume:
23
Issue:
56
Pages:
14080–14089
Publication date:
2017-09-08
Acceptance date:
2017-08-01
DOI:
ISSN:
1521-3765
Source identifiers:
713283
Language:
English
Keywords:
Pubs id:
pubs:713283
UUID:
uuid:f33ab4c4-22b3-4443-9efe-5d038e884be4
Local pid:
pubs:713283
Deposit date:
2017-08-11

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