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An experimental study of OH(A(2)Σ(+)) + H2: Electronic quenching, rotational energy transfer, and collisional depolarization

Abstract:

Zeeman quantum beat spectroscopy has been used to determine the thermal (300 K) rate constants for electronic quenching, rotational energy transfer, and collisional depolarization of OH(A(2)Σ(+)) by H2. Cross sections for both the collisional disorientation and collisional disalignment of the angular momentum in the OH(A(2)Σ(+)) radical are reported. The experimental results for OH(A(2)Σ(+)) + H2 are compared to previous work on the OH(A(2)Σ(+)) + He and Ar systems. Further comparisons are al...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1063/1.4989567

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Institution:
University of Oxford
Oxford college:
Jesus College
Role:
Author
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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
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Funding agency for:
Brouard, M
Grant:
FP7 EU People ITN Project No. 238671
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Funding agency for:
Brouard, M
Grant:
FP7 EU People ITN Project No. 238671
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Grant:
to M.B. via FP7 EU People ITN Project No. 238671
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Grant:
to F.J.A. via the No. CTQ2015-65033-P (MINECO/FEDER) grant
Publisher:
AIP Publishing Publisher's website
Journal:
Journal of Chemical Physics Journal website
Volume:
146
Issue:
24
Article number:
244313
Publication date:
2017-06-28
Acceptance date:
2017-06-09
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
Source identifiers:
708028
Language:
English
Pubs id:
pubs:708028
UUID:
uuid:fe748146-7f03-43a1-8cac-be36dfa1ae45
Local pid:
pubs:708028
Deposit date:
2017-07-14

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